Adelaide Research & Scholarship
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https://hdl.handle.net/2440/34911
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| Type: | Journal article |
| Title: | Delocalizing Electrons in Water with Light |
| Author: | Son, D. Kambhampati, P. Kee, T. Barbara, P. |
| Citation: | The Journal of Physical Chemistry A: Isolated Molecules, Clusters, Radicals, and Ions; Environmental Chemistry, Geochemistry, and Astrochemistry; Theory, 2001; 105(36):8269-8272 |
| Publisher: | Amer Chemical Soc |
| Issue Date: | 2001 |
| ISSN: | 1089-5639 1520-5215 |
| Statement of Responsibility: | Dong Hee Son, Patanjali Kambhampati, Tak W. Kee, and Paul F. Barbara |
| Abstract: | Experimental information on the spatial extent of the putative p and conduction band states of the hydrated electron (eeq) has been obtained by monitoring and controlling the electron/hole spatial separation of a photogenerated eeq/hole pair using a femtosecond laser pulse sequence. Optical excitation of eeq with two photons is observed to dramatically alter its spatial distribution and geminate recombination yield with the hole. One-photon excitation, in contrast, has no effect on the spatial distribution. The results strongly confirm theoretical predictions on the size and location of excited states of eeq. |
| Description: | © Copyright 2001 by the American Chemical Society |
| DOI: | 10.1021/jp012431p |
| Published version: | http://pubs.acs.org/cgi-bin/abstract.cgi/jpcafh/2001/105/i36/abs/jp012431p.html |
| Appears in Collections: | Aurora harvest 6 Chemistry publications Environment Institute publications |
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